This dataset is a model output from the European Monitoring and Evaluation Programme (EMEP) model applied to the UK (EMEP4UK) driven by Weather and Research Forecast model meteorology (WRF). It provides annual total atmospheric deposition of cadmium, copper, nickel, lead, zinc, sulphur, and nitrogen over the UK on a 3x3 km2 grid for years between 1750 and 2018. The EMEP4UK model version used here is rv4.36, and the WRF model version is the 4.2.2. This work was supported by the Natural Environment Research Council award number NE/R016429/1 as part of the UK-SCAPE programme delivering National Capability.